Being a caregiver can be very trying on the patience. Remember he is probably more upset about loosing his independence or not being able to do the small things himself. Try not to take anything personal, and go in with the mindset of "how would I feel if I were in his shoes".
Here is a list of things to ask the Lord for. It may be an idea to include your grandfather while praying these scriptures as well.
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mso-style-priority:99; mso-style-parent:""; mso-padding-alt:0in 5.4pt 0in 5.4pt; mso-para-margin-top:0in; mso-para-margin-right:0in; mso-para-margin-bottom:10.0pt; mso-para-margin-left:0in; line-height:115%; mso-pagination:widow-orphan; font-size:11.0pt; font-family:"Calibri","sans-serif"; mso-ascii-font-family:Calibri; mso-ascii-theme-font:minor-latin; mso-hansi-font-family:Calibri; mso-hansi-theme-font:minor-latin; mso-bidi-font-family:"Times New Roman"; mso-bidi-theme-font:minor-bidi;} </style> <![endif]--> Anah (Lord to hear) Psa 119:145
Natsar(keep Lord’s statutes, testimonies) Psa 119:145
Yachel (be patient, hope) Psa 119:147
Chesed(lovingkindness) Psa110:149
Chayah (quicken, restore) Psa 119:149
Chalats (deliver) Psa 119:153
Riyb (Christ to plead cause) Psa 119:154
Racham (tender mercy) Psa 119:156
Pachad (stand in awe of God’s Word) Psa 119:161
Sus (rejoice) Psa 119: 162
Halal (praise Lord) Psa 119:164
Shalom(peace) Psa 119:165
Ayin Mikshol (nothing to offend) Psa 119:165
Lamad(teach) Psa 119:171